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Green Conversion of Spent Lithium-Ion Batteries via Infrared Pyrolysis: Gas-Assisted Metal Recovery and Reaction Pathway Elucidation
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC05022G, PaperMoshan Li, Zuohua Liu, Erfeng Hu, Guangwen Xu, Rui Qu, Jianglong Yu, Dean Pan, Youcai Ma
The recycling of waste lithium-ion batteries (LIBs) plays a pivotal role in the sustainable advancement of renewable energy technologies. This study presented a new technique for ex-situ recovery of cobalt...
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DOI: 10.1039/D5GC05022G, PaperMoshan Li, Zuohua Liu, Erfeng Hu, Guangwen Xu, Rui Qu, Jianglong Yu, Dean Pan, Youcai Ma
The recycling of waste lithium-ion batteries (LIBs) plays a pivotal role in the sustainable advancement of renewable energy technologies. This study presented a new technique for ex-situ recovery of cobalt...
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Electrochemical sulfonylation with sulfur dioxide: a sustainable strategy for organic synthesis
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC04193G, Tutorial ReviewZhi-Long Lei, Hai-Tao Tang, Ying-Ming Pan
The utilization of organic electrochemical methods to achieve efficient and green conversion and fixation of sulfur dioxide (SO₂) has become a highly attractive research direction in the field of organic...
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DOI: 10.1039/D5GC04193G, Tutorial ReviewZhi-Long Lei, Hai-Tao Tang, Ying-Ming Pan
The utilization of organic electrochemical methods to achieve efficient and green conversion and fixation of sulfur dioxide (SO₂) has become a highly attractive research direction in the field of organic...
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In-Situ Reduction Engineering of NiFe-NiFe 2 O 4 Heterojunctions for Interfacial Coupling toward Efficient Bifunctional Zinc-Air Batteries
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC04845A, PaperYi Hu, Ning Han, Yiting Wu, Cong Han, Lizi He
Single-component catalysts face inherent challenges in striking a balance between the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER) due to their sluggish kinetics and divergent reaction requirements....
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DOI: 10.1039/D5GC04845A, PaperYi Hu, Ning Han, Yiting Wu, Cong Han, Lizi He
Single-component catalysts face inherent challenges in striking a balance between the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER) due to their sluggish kinetics and divergent reaction requirements....
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Trace-LiCl-assisted synthesis of high-loading ordered Pt3Co intermetallic catalysts for the oxygen reduction reaction in fuel cells
DOI: 10.1039/D5GC05077D, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Yutao Ni, Jiahui Song, Huiying Lan, Xue Jing, Wenwen Shi, Ruimin Ding, Xi YinUnderstanding the synthesis mechanism of Pt3Co guided the development of high-loading Pt3Co catalysts assisted by trace LiCl, which demonstrated high efficiency in proton exchange membrane fuel cells.
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Following forest cues for the harvest optimization of tomorrow's biofeedstocks
DOI: 10.1039/D5GC04279H, Paper
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Robyn C. O'Halloran, Alison J. Shapiro, Yagya Gupta, Anna Long, Sara G. Haney, Yuichiro Otsuka, Sunitha Sadula, Dionisios G. Vlachos, Delphis F. Levia, Thomas H. EppsHarvest optimization offers an effective strategy for maximizing lignin valorization yields and overall biorefinery production of fuels, chemicals, and materials.
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Site-selective electrochemical C(sp3)–H late-stage functionalization of pyrazolones
DOI: 10.1039/D5GC02947C, CommunicationJing-Yi Zhang, Ming-Han Li, Yu-Shun Cui, Ying Yang, Miao Lai, Zi-Xun Gao, Lin-Yu Zheng, Si-Ao Lu, Bin-Tao Liu, Fang-Ling Lu, Yu-Lin Feng
A cost-effective and sustainable electrochemical strategy enables highly selective C(sp3)–H functionalization of pyrazolones. 116 valuable novel pyrazolone derivatives were rapidly synthesized under mild conditions.
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A feasible methanol economy for a green future
DOI: 10.1039/D5GC04615G, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Hidde Kolmeijer, Abhinandan Nabera, Antonio J. Martín, Gonzalo Guillén-Gosálbez, Javier Pérez-RamírezThis study models a future methanol economy where combining biomass, biogas, and air-captured CO2 achieves net-zero emissions at about 32 USD2025 per person per month, close to Paris Agreement-aligned costs while delivering deeper emission cuts.
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Degradable polymer films: RAFT-mediated emulsion copolymerization of lipoic acid with vinyl monomers
DOI: 10.1039/D5GC04609B, Paper
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Steven W. Thompson, Yasemin Fadil, Nicholas J. Chan, Graeme Moad, Sébastien Perrier, Per B. ZetterlundLipoic acid (LA) was successfully incorporated in PBA-b-PSt diblock copolymers via RAFT emulsion polymerization. Films were formed with LA showing minimal effect on mechanical properties. Degradation in DMF results in large molecular weight decrease.
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Photoinduced carbonylative synthesis of β-trifluoromethylated thioesters through 1,2-trifluoromethylation and carbonylation of alkenes
DOI: 10.1039/D5GC04881H, Communication
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Ren-Guan Miao, Zhi-Peng Bao, Yuanrui Wang, Chang-Sheng Kuai, Xiao-Feng WuA novel visible light-induced metal-free carbonylation method for the synthesis of β-trifluoromethylated thioesters has been developed.
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Tunable stereoselectivity in a wireless electrochemical microreactor using natural chiral ionic liquids
DOI: 10.1039/D5GC04756K, Communication
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Sara Grecchi, Andrea Mezzetta, Lorenzo Guazzelli, Serena ArnaboldiA green and sustainable enantioselective electrosynthesis strategy using a drop of naturally derived chiral ionic liquid, harnessed within a polypyrrole tube microreactor acting as an efficient wireless pump.
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NiFe-LDH loaded on N-doped Paulownia-derived carbon as a bifunctional oxygen electrocatalyst for rechargeable zinc–air batteries
DOI: 10.1039/D5GC03239C, PaperNing Duan, Pengxiang Zhang, Xiaofeng Zhang, Pan Li, Xianli Wu, Yanyan Liu, Guosheng Han, Baojun Li
2D NiFe-LDH nanosheets loaded on 3D N-doped biomass-derived carbon, NiFe-LDH/NBC, were prepared using an in situ growth method assisted by electric field induction as an excellent bifunctional electrocatalytic catalyst.
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Single-atom iron-anchored graphitic C3N5 for photocatalytic trifluoromethylation of aromatics and N-heterocycles in water
DOI: 10.1039/D5GC03873A, PaperXiaolong Li, Xueping Zhang, Mei Hong, Weihao Zhou, Yamei Lin, Guo-Ping Lu
Anchoring single-atom Fe on g-C3N5 creates a green, efficient strategy for aqueous trifluoromethylation. This recyclable photocatalyst synthesizes fluorinated compounds while avoiding toxic solvents and metal waste.
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Pore -tailored hollow mesoporous carbon spheres confined with Pd/PdO nanoparticles enable the coupling of efficient CO2 reduction and propylene oxidation
DOI: 10.1039/D5GC04779J, PaperMan Zhao, Ze Wang, Jiamin Ma, Qinyun Yan, Liwu Qiang, Wei Wen, Lifang Shi, Shuai He, Na Gao, Aiqin Hao, Junming Zhang, Xiaoli Li, He Xiao, Jianfeng Jia
Schematic of CO2RR over Pd/HMCs-10 and POR over PdO/HMCs-10 in a coupled catalytic system, showing the effect of particle size of Pd NPs in Pd/HMCs-x on the CO2RR activity and PdO NPs in PdO/HMCs-x on the POR activity.
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Green upcycling of retired asphalt into “vortex-crosslinked” carbon anodes for high-performance sodium-ion batteries
DOI: 10.1039/D5GC05322F, PaperDanqing Li, Xin He, Linlin Wang, Mei Ding, Chunhui Gao, Chuankun Jia
The environmental burden of waste asphalt and the performance limitations of sodium-ion battery anodes pose dual challenges in energy and sustainability.
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Continuous-flow synthesis of organic urea derivatives from CO2-absorbed alkanolamines over a CeO2 catalyst
DOI: 10.1039/D5GC05210F, PaperShogen Mihara, Natsuki Mizutani, Hikari Terada, Mizuho Yabushita, Takaaki Endo, Yoshinao Nakagawa, Akira Nakayama, Keiichi Tomishige
Continuous conversion of CO2-absorbed alkanolamines in the corresponding amine solvent was demonstrated with a fixed-bed flow reactor and a CeO2 catalyst. Both the reaction rate and pathway were governed by the alkyl chain length of alkanolamines.
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Molecular property prediction for very large databases with natural language processing: a case study in ionic liquid design
DOI: 10.1039/D5GC02803E, Paper
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Mood Mohan, Michelle K. Kidder, Jeremy C. SmithHerein, we report the development of machine learning models for predicting the properties of ionic liquids using Mol2vec featurization technique and this approach enables accelerated development of ILs with optimal properties.
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Towards sustainable plastics: a sustainable chemistry assessment
DOI: 10.1039/D5GC03504J, PaperJiazhe Chen, Zhichun Zhang, Qiaonan Jing, Shaoxuan Zhang, Rongjing Lu, Jianguo Liu
A transition from conventional linear plastic lifecycle to clean circular economy: minimize chemical footprint, accelerate plastic circularity, and promote low-carbon process.
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Fully liquid electrorefining: a highly efficient and selective approach for pure lithium metal recovery from low-grade alloys
DOI: 10.1039/D5GC02624E, PaperYuntao Lei, Wenjuan Zhang, Fenglong Sun, Zhongwei Zhao
High-purity lithium metal is extracted from alloy feedstocks with high selectivity and efficiency via a fully liquid electrorefining system.
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Mechanism-controlled switchable regioselective O- and N-cyclization alkenylation of alkenylbenzamides via dual photoredox and cobalt catalysis
DOI: 10.1039/D5GC04510J, PaperFeiyang Rao, Kui Hu, Yuanxiang He, Ziyi Zuo, Shiming Lv, Shu Geng, Li Pan, Hongmei Wang, Feng Huang
By regulating the redox potential matching between the substrate active sites and photocatalytic systems to control the reaction pathway, this approach achieves switchable regioselective O- and N-cyclization alkenylation of alkenylbenzamides.
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Porphyrin and phthalocyanine-based covalent organic frameworks for electrocatalytic CO2 reduction: from structural design to future perspectives
DOI: 10.1039/D5GC04855A, Tutorial ReviewYaoqian Feng, Ning Huang
The electrocatalytic CO2 reduction reaction (ECO2RR) offers a sustainable route for converting CO2 into high-value-added chemicals and fuels, presenting a viable solution to urgent energy and environmental issues.
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