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Bi-doped directional spin-polarised electron injection modulates MBene surface d–d coupling to promote nitrogen reduction kinetics
DOI: 10.1039/D5GC04584C, PaperKun Cheng, Shaobin Li, Qingyu Cheng, Li Zhang, Yufeng Jiang, Fengbo Li, Xiaoqing Lv
Bi doping modulates Fe 3d orbital spin, directionally injecting electrons into Mo via d–d hybridization to adjust the Mo d-band center, enhancing ambient electrocatalytic nitrogen fixation for MBene heterostructure.
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Chemically recyclable, fully biobased polyolefins with performance parity to low-density polyethylene
DOI: 10.1039/D5GC05344G, PaperWei Sun, Yuzhe Pang, Yucheng He, Zhenyang Luo, Puyou Jia, Yonghong Zhou, Ye Sha
We demonstrate a homopolymerization strategy for the controlled synthesis of fully biobased, high-molecular-weight polyolefins. These materials exhibit thermomechanical properties comparable to LDPE while being chemically recyclable.
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Avoiding tomorrow's chemical mistakes today
DOI: 10.1039/D5GC05283A, Perspective
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Jeroen B. Guinée, Martina G. VijverAdvancing SSbD requires an effective and efficient regulatory-based data strategy to improve data availability and quality for safety assessments and LCA; without it, new methods may merely become empty promises that avoid the real issue.
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Lithium extraction from spinel LiMn2O4 with simultaneous preparation of λ-MnO2 under mild conditions using sodium hypochlorite
DOI: 10.1039/D5GC04585A, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Yanhui Kong, Yutaro Takaya, Mauricio Córdova-Udaeta, Chiharu TokoroLithium extraction from spinel LiMn2O4 is important because it is both a mainstream LIB cathode and a key precursor for λ-MnO2, which is widely used for selective lithium extraction from brines and seawater.
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The catalytic conversion of fructose to difructose anhydride
DOI: 10.1039/D5GC04714E, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Isabel Hortal-Sánchez, Faysal Ibrahim, Edgard A. Lebrón-Rodríguez, Fabiola Y. Rodríguez-Rodríguez, Grace Gooley, Ruining Ma, Matias Alvear, Ive Hermans, Nelson Cardona-MartínezThe production of difructose anhydride (DFA) from fructose under mild conditions, in a green/bio-derived solvent. Crystal structure created with VESTA, J. Appl. Crystallogr., 2011, 44, 1272–1276.
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Metal-free stereoselective C(sp3)–H indolation of N-heterocycles to potent antimicrobial non-canonical tryp–pro hybrids
DOI: 10.1039/D5GC04622J, PaperSubhajit Saha, Soumya Ranjan Bag, Abdul Akhir, Deepanshi Saxena, Rahul Maitra, Sidharth Chopra, Chandan K. Jana
Direct diastereoselective C–H indolations of N-heterocycles under metal and oxidant-free conditions have been developed for one-step access to enantioenriched indolyl N-heterocycles as new antibacterial scaffolds against multidrug-resistant strains.
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An applied machine learning framework for waste lithium-ion battery leaching with integrated preliminary environmental and economic assessment
DOI: 10.1039/D5GC04752H, PaperAndré Nogueira, Filipe H. B. Sosa, Ana C. Dias, João A. P. Coutinho, Nicolas Schaeffer
Data-driven LIB recycling: a new ML framework predicts metal leaching yields and evaluates process sustainability through integrated economic and environmental impact assessments.
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Polyetherureas as aqueous binders for Li ion batteries
DOI: 10.1039/D5GC03953C, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Garima Saini, Mei Jun Tan, Maximillian G. Stanzione, Ketan Pancholi, Harini Sampathkumar, Matthew Walker, Charlie Patterson, Massimo Vassalli, Aaron B. Naden, Oxana V. Magdysyuk, Jiyu Tian, A. Robert Armstrong, Amit KumarThis study presents polyetherureas, synthesized via a green, diisocyanate-free route, as a novel aqueous binder for LiFePO4 cathodes in lithium-ion batteries, showing comparable performance to conventional CMC binders. Image created partly using Google Gemini.
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An electrochemically promoted modular synthesis of diverse glycomimetics via acyloxyphosphonium ions
DOI: 10.1039/D5GC04739K, PaperYi-Min Jiang, Cheng-Lin Ding, Guizhen Zhang, Hongbao Sun, Jie Liu
A mild, modular electrochemical method constructs glycomimetics by linking sugars to target molecules. This iodine-mediated, metal- and oxidant-free strategy features a broad substrate scope for efficient bioactive compound synthesis.
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A green and efficient strategy for leaching critical metals from spent LiNixCoyMnzO2 cathodes: modulating the dielectric SiO2 contact-electro-catalytic activity
DOI: 10.1039/D5GC04080A, PaperMan Yang, Shuhao Qin, Youchang Yang, Mingmi Wu, Ting Lei, Yufei Liu, Huiju Shao
This work developed a CEC-leaching process for efficient and eco-friendly recycling of spent LIB cathodes, which avoids secondary pollution, reduces energy and reagent consumption, and aligns with green chemistry and circular economy principles.
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Electrochemical metal-free functionalization of ArCF3: efficient construction of C–S, C–Se, C–D, C–H, and C–C bonds
DOI: 10.1039/D5GC05060J, CommunicationZhimin Xu, Zonghao Zhou, Xiaochen Wang, Yuxia Yang, Yi Pan, Yi Wang
A strategy for electrochemical defluorinative functionalization of ArCF3 is presented, providing access to C–S, C–Se, C–H, C–D, and C–C bonds.
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Photocatalytic upcycling of PET into methane, hydrogen and high-value liquid products
DOI: 10.1039/D5GC03562G, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Madeline Weisweiller, Adrian Ertl, Cornelia von Baeckmann, Anil Kumar Sihag, Christian M. Pichler, Freddy Kleitz, Dominik Eder, Alexey CherevanWe systematically study the key process parameters of polyethylene terephthalate (PET) microplastic photoreforming. We uncover that not only hydrogen (H2) but also methane (CH4) is generated and provide valuable mechanistic insights into the process.
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Si-doped γ-Al2O3 from solid-phase grinding for highly efficient one-step production of L,L-lactide
DOI: 10.1039/D5GC04167H, PaperMin-Min Wang, Hong Guo, Zheng-Wu Wang, Yu-Quan Yan, Yi-Zhou Zhu, He-Fang Wang
A new SPG-Si-Al2O3 catalyst made from a simple and easily-scaled-up strategy of solid-phase grinding achieves one-step high-efficiency conversion of lactic acid to lactide.
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A multi-enzyme cascade coupled with electrochemistry for efficient synthesis of L-lactate from carbon dioxide
DOI: 10.1039/D5GC05391A, PaperShanquan Liang, Zhiyao Peng, Xue Xia, Kaixing Xiao, Zhao Qin, Xuemei Liu, Fanzhen Lin, Mengdie Wang, Saimeng Jin, James H. Clark, Dan Wang
An electro-enzymatic coupling platform was established by coupling the multi-enzyme cascade system with electrochemistry for effective regeneration of NADH to produce L-lactate.
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Linear paired electrolysis enabled dearomative [3 + 2] cycloadditions of indoles and benzofurans with vinyl azides
DOI: 10.1039/D5GC04148A, PaperShaoxiong Yang, Yanren Zhu, Enfan Pu, Piaopiao Jiang, Xiong Li, Hongbin Zhang, Jingbo Chen
We report an efficient protocol for dearomative [3 + 2] cycloadditions of indoles and benzofurans with vinyl azides via linear paired electrolysis under redox-neutral conditions.
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Photoredox Catalysis with Pyridinium and Structurally Related Onium Salts: Sustainable Synthesis via Reactive Oxygen Species and Electron Transfer
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03738G, Tutorial ReviewXin-Rong Yao, Jing-Wang Cui, Meng-Ze Jia, Jie Zhang
Pyridinium and its derivatives, which incorporate both redox centers and Lewis acid sites, exhibit high structural tunability. Their excited states can generate singlet oxygen via energy transfer or undergo electron...
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DOI: 10.1039/D5GC03738G, Tutorial ReviewXin-Rong Yao, Jing-Wang Cui, Meng-Ze Jia, Jie Zhang
Pyridinium and its derivatives, which incorporate both redox centers and Lewis acid sites, exhibit high structural tunability. Their excited states can generate singlet oxygen via energy transfer or undergo electron...
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Carrier-free silver carbonate catalysis: In situ conversion of low concentration CO2 in air and actual exhaust gas to oxazolidinones
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC04212G, CommunicationPei-Bo Chen, Wang Chen, Jia-Wen Yang, Chan-Cui Wu, Hai-Tao Tang, Ying-Ming Pan, Ying Liang
The increasing concentration of CO₂ in the atmosphere drives global climate change, and efficient methods for CO₂ utilisation are urgently needed. This study introduces a novel carrier-free catalytic approach using...
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DOI: 10.1039/D5GC04212G, CommunicationPei-Bo Chen, Wang Chen, Jia-Wen Yang, Chan-Cui Wu, Hai-Tao Tang, Ying-Ming Pan, Ying Liang
The increasing concentration of CO₂ in the atmosphere drives global climate change, and efficient methods for CO₂ utilisation are urgently needed. This study introduces a novel carrier-free catalytic approach using...
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Sustainable bubble-mediated dynamic triphasic antisolvent crystallization for magnesium sulfate nano-micron particles: Precise size and morphology control
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC05730B, PaperYingchen Wang, Sheng Liu, Jiaqi Luo, Mingting Yuan Yuan, Yimin Jia, Qiutong Zhang, Wenhao Yan, Qiushuo Yu
Particle ultrafine processing is an effective strategy for enhancing the physical and chemical properties of materials. However, traditional antisolvent crystallization for ultrafine particle preparation often faces the challenge of uneven...
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DOI: 10.1039/D5GC05730B, PaperYingchen Wang, Sheng Liu, Jiaqi Luo, Mingting Yuan Yuan, Yimin Jia, Qiutong Zhang, Wenhao Yan, Qiushuo Yu
Particle ultrafine processing is an effective strategy for enhancing the physical and chemical properties of materials. However, traditional antisolvent crystallization for ultrafine particle preparation often faces the challenge of uneven...
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From Lignin to Jet Fuel: Advancing Selective Cyclohydrocarbon Production Toward Full Compatibility with Aviation Standards
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC04813C, Tutorial Review Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Jianyu Wang, Zheng Li, Chun Zhao, Jing Zhang, Aiguo Wang, Liquan Jing, Na Zhong, Zhangxin Chen, Jinguang Hu
Sustainable aviation fuel (SAF) derived from lignocellulosic biomass represents a critical pathway to decarbonizing the aviation sector. As the only abundant, naturally aromatic biopolymer, lignin offers unique potential for producing...
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DOI: 10.1039/D5GC04813C, Tutorial Review
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Jianyu Wang, Zheng Li, Chun Zhao, Jing Zhang, Aiguo Wang, Liquan Jing, Na Zhong, Zhangxin Chen, Jinguang HuSustainable aviation fuel (SAF) derived from lignocellulosic biomass represents a critical pathway to decarbonizing the aviation sector. As the only abundant, naturally aromatic biopolymer, lignin offers unique potential for producing...
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Strategic Sodium Modulation for Low-Temperature Fabrication of Phase-Pure Na 3 V 2 (PO 4 ) 3 Cathodes: Mechanistic Insights and Performance Optimization in Sodium-Ion Batteries
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC05076F, PaperZhaojin Li, Yunbo Di, Zhicheng Wang, Di Zhang, Huilan Sun, Qujiang Sun, Qiujun Wang, Fei Yuan, Ranran Li, Bo Wang
The synthesis of high-purity Na3V2(PO4)3 (NV2P) cathodes is persistently challenged by the formation of Na3V3(PO4)4 (NV3P) impurities and energy-intensive high-temperature processing (>800 °C), which promotes phosphate decomposition and detrimental grain...
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DOI: 10.1039/D5GC05076F, PaperZhaojin Li, Yunbo Di, Zhicheng Wang, Di Zhang, Huilan Sun, Qujiang Sun, Qiujun Wang, Fei Yuan, Ranran Li, Bo Wang
The synthesis of high-purity Na3V2(PO4)3 (NV2P) cathodes is persistently challenged by the formation of Na3V3(PO4)4 (NV3P) impurities and energy-intensive high-temperature processing (>800 °C), which promotes phosphate decomposition and detrimental grain...
The content of this RSS Feed (c) The Royal Society of Chemistry