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Visible light-driven regioselective tert-butyl peroxidation and hydroperoxidation of alkenes with TBHP
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02911B, PaperRenhua Su, Jiantao Zhang, Yanfu Jiang, Xian Jiang, Peng Zhou, Jingxing Jiang, Weibing Liu
We reported a visible-light-driven, photocatalyst-free bisperoxidation of aryl alkenes with tert-butyl hydroperoxide (TBHP), enabling the regioselective synthesis of α,β-bisperoxides. To our knowledge, this represents the first radical reaction utilizing TBHP...
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DOI: 10.1039/D5GC02911B, PaperRenhua Su, Jiantao Zhang, Yanfu Jiang, Xian Jiang, Peng Zhou, Jingxing Jiang, Weibing Liu
We reported a visible-light-driven, photocatalyst-free bisperoxidation of aryl alkenes with tert-butyl hydroperoxide (TBHP), enabling the regioselective synthesis of α,β-bisperoxides. To our knowledge, this represents the first radical reaction utilizing TBHP...
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Biobased amide surfactants derived from cellulose–waste hydroxy acids: mechanochemical synthesis, foam fractionation and performance
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01806D, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Giorgia Crigna, Davide Moscatelli, Tuomo Sainio
A series of hydroxycarboxylic acids (HAs) with excellent hydrophilic properties are produced from alkali treatment of cellulose–containing materials. The great majority of these hydroxy acids is constituted by glucoisosaccharinic acids...
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DOI: 10.1039/D5GC01806D, Paper


A series of hydroxycarboxylic acids (HAs) with excellent hydrophilic properties are produced from alkali treatment of cellulose–containing materials. The great majority of these hydroxy acids is constituted by glucoisosaccharinic acids...
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Intramolecular Nitrogen Insertion of Oxime Ester access to Aminated N-heterocycles
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02482J, CommunicationHan Wang, Jing Feng, Dan-Ni Liu, Mingming Yu, Ze-Feng Xu, Chuan-Ying Li
The synthesis of aminated N-heterocycles is a critical area in organic synthetic chemistry. But some issues need to be addressed for traditional amination of N-heterocycles, such as the need of...
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DOI: 10.1039/D5GC02482J, CommunicationHan Wang, Jing Feng, Dan-Ni Liu, Mingming Yu, Ze-Feng Xu, Chuan-Ying Li
The synthesis of aminated N-heterocycles is a critical area in organic synthetic chemistry. But some issues need to be addressed for traditional amination of N-heterocycles, such as the need of...
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Efficient and Low-Carbon Synthesis of Colorless Transparent Polyimides
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01983D, PaperJiahui Liu, Chuying Li, Yanwei He, Bo Deng, Haitao Huang, Siwei Liu, Yi Zhang
The widespread use of polyimide varnish in semiconductors, packaging, and flexible displays has created increasing demand for efficient and environmentally friendly preparation. Compared to polyamic acid varnish, polyimide varnish offers...
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DOI: 10.1039/D5GC01983D, PaperJiahui Liu, Chuying Li, Yanwei He, Bo Deng, Haitao Huang, Siwei Liu, Yi Zhang
The widespread use of polyimide varnish in semiconductors, packaging, and flexible displays has created increasing demand for efficient and environmentally friendly preparation. Compared to polyamic acid varnish, polyimide varnish offers...
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Ionic Liquid-Mediated Hydrogen-Bond Network: A Pathway to High-Efficiency PEMFCs with Unlocked Active Sites of Pt/C catalysts
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01820J, PaperMiao Ma, Lixiao Shen, Pan Guo, Bo Liu, Ziyu Zhang, Yunfei Xia, Zigang Zhao, Aibing Chen, Yunlong Zhang, Lei Zhao, Zhenbo Wang
The strong adsorption of ionomer sulfonate groups (-SO3-) onto platinum (Pt) nanoparticles significantly hinders the catalytic activity and mass transport at the Pt/ionomer interface, compromising electrode reaction efficiency in proton...
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DOI: 10.1039/D5GC01820J, PaperMiao Ma, Lixiao Shen, Pan Guo, Bo Liu, Ziyu Zhang, Yunfei Xia, Zigang Zhao, Aibing Chen, Yunlong Zhang, Lei Zhao, Zhenbo Wang
The strong adsorption of ionomer sulfonate groups (-SO3-) onto platinum (Pt) nanoparticles significantly hinders the catalytic activity and mass transport at the Pt/ionomer interface, compromising electrode reaction efficiency in proton...
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Assessing Mass Intensity as a Green Chemistry Metric: Why Expanding System Boundaries is not Enough
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02994E, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Stefan Eichwald, Hesam Ostovari, Hannah Minten, Janine Meyer-Waßewitz, Dieter Förtsch, Niklas von der Assen
Evaluating the environmental impacts of chemicals is crucial for a sustainable chemical industry. While Life Cycle Assessment (LCA) is recommended for evaluating environmental impacts, collecting chemical life-cycle data is often...
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DOI: 10.1039/D5GC02994E, Paper


Evaluating the environmental impacts of chemicals is crucial for a sustainable chemical industry. While Life Cycle Assessment (LCA) is recommended for evaluating environmental impacts, collecting chemical life-cycle data is often...
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One-Pot Electrocatalytic Lignin Depolymerization with In-Situ Extraction: A Feasible Approach Toward Biomass-Based Oils
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01810B, PaperLucie M. Lindenbeck, Silas Brand, Finn Schatz, Franka Stallmann, Nele Petersen, Björn B. Beele, Jessica Pichler, Marcella Frauscher, Raphaela Süss, Pascal Olschowski, Serhiy Budnyk, Adam Slabon, Bruno V.M. Rodrigues
This investigation presents a one-pot electrochemical depolymerization of lignin, coupled with in-situ extraction, to enhance product recovery and process efficiency. Kraft lignin was dissolved in an aqueous sodium carbonate solution...
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DOI: 10.1039/D5GC01810B, PaperLucie M. Lindenbeck, Silas Brand, Finn Schatz, Franka Stallmann, Nele Petersen, Björn B. Beele, Jessica Pichler, Marcella Frauscher, Raphaela Süss, Pascal Olschowski, Serhiy Budnyk, Adam Slabon, Bruno V.M. Rodrigues
This investigation presents a one-pot electrochemical depolymerization of lignin, coupled with in-situ extraction, to enhance product recovery and process efficiency. Kraft lignin was dissolved in an aqueous sodium carbonate solution...
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Dynamic Solvent System as a novel approach to sustainable MOF crystallization.
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01029B, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Leonid Shupletsov, Alina Christin Schieck, Irena Senkovska, Volodymyr Bon, Stefan Kaskel
Herein we report a novel and green synthetic approach for pyrazolate-based metal-organic frameworks (MOFs) as demonstrated by the three prominent examples of this material class: [Ni(bdp)]n, and two supramolecular isomers...
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DOI: 10.1039/D5GC01029B, Paper


Herein we report a novel and green synthetic approach for pyrazolate-based metal-organic frameworks (MOFs) as demonstrated by the three prominent examples of this material class: [Ni(bdp)]n, and two supramolecular isomers...
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Trifluoromethanesulfinyl chloride: An effective trifluoromethyl radical source in the trifluoromethylimination of alkenes
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01651G, CommunicationWeilong Lin, Jiayu Liang, Shuping Wang, Xingda Zhao
The trifluoromethyl (CF3) group has emerged as a privileged structural motif in pharmaceutical compounds and biologically active molecules, leading to a significant demand for efficient synthetic methodologies to incorporate the...
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DOI: 10.1039/D5GC01651G, CommunicationWeilong Lin, Jiayu Liang, Shuping Wang, Xingda Zhao
The trifluoromethyl (CF3) group has emerged as a privileged structural motif in pharmaceutical compounds and biologically active molecules, leading to a significant demand for efficient synthetic methodologies to incorporate the...
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Porous liquids for gas capture and separation: recent progress and future aspects
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03111G, Critical ReviewLisha Sheng, Hailong Ning, Yi Wang, Chengyi Li, Shengtao Huang, Yuquan Zhang, Bo Xu, Zhenqian Chen
Porous liquids are a novel class of porous materials, which integrate the permanent porosity of solids with the fluidity of liquids. By rational combination of the porous solids and liquid...
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DOI: 10.1039/D5GC03111G, Critical ReviewLisha Sheng, Hailong Ning, Yi Wang, Chengyi Li, Shengtao Huang, Yuquan Zhang, Bo Xu, Zhenqian Chen
Porous liquids are a novel class of porous materials, which integrate the permanent porosity of solids with the fluidity of liquids. By rational combination of the porous solids and liquid...
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Organic-electrical reduction of carbon-carbon double bonds
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01804H, Tutorial ReviewBao-Jie Wang, Yi-Le Song, Ke Li, Li-Rong Wen, Ming Li, Jiaxiu Liu, Weisi Guo, Lin-Bao Zhang
Organic electrochemical synthesis has become a practical and environmentally friendly synthesis method, widely used in oxidation, reduction, and redox-neutral reactions. By precisely controlling the current or potential, it is possible...
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DOI: 10.1039/D5GC01804H, Tutorial ReviewBao-Jie Wang, Yi-Le Song, Ke Li, Li-Rong Wen, Ming Li, Jiaxiu Liu, Weisi Guo, Lin-Bao Zhang
Organic electrochemical synthesis has become a practical and environmentally friendly synthesis method, widely used in oxidation, reduction, and redox-neutral reactions. By precisely controlling the current or potential, it is possible...
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Renewable Energy-Driven Synthesis of Bioactive Quinolinones through Photocatalytic and Electrochemical Activation
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02521D, CommunicationQingge Zhao, Mengyu Peng, Huimin Li, Longqiang Zhao, Xinyue Song, Peiyao Zhao, Shoucai Wang, Guangbin Jiang, Fanghua Ji
We present an innovative photocatalytic system for sustainable quinolin-2(1H)-one synthesis with broad substrate scope under mild, oxidant-free conditions, overcoming limitations of harsh traditional methods and high-pressure CO dependency. A complementary...
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DOI: 10.1039/D5GC02521D, CommunicationQingge Zhao, Mengyu Peng, Huimin Li, Longqiang Zhao, Xinyue Song, Peiyao Zhao, Shoucai Wang, Guangbin Jiang, Fanghua Ji
We present an innovative photocatalytic system for sustainable quinolin-2(1H)-one synthesis with broad substrate scope under mild, oxidant-free conditions, overcoming limitations of harsh traditional methods and high-pressure CO dependency. A complementary...
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Toughened commercial poly(L-lactide) (PLLA) using degradable and recyclable poly(ester-alt-ether)-b-PLLA
DOI: 10.1039/D5GC02301G, Paper


Properties of bio-derived poly(L-lactide) are improved by block polymer additives which deliver efficient chemical recycling and enzymatic hydrolysis. Blends compete with poly(acrylonitrile-butadiene-styrene) and high impact polystyrene.
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Innovative bacterial cellulose and UiO-66 composites for superior zinc ion battery separator performance
DOI: 10.1039/D5GC01051A, PaperTian Zhao, Pengcheng Xiao, Saiqun Nie, Jiangrong Yu, Shilin Peng, Jiayao Chen, Fuli Luo, Yi Chen
Pure BC separator lack channels, causing loose Zn2+ deposition and dendrites. In situ UiO-66 growth on BC forms hierarchical pores for uniform Zn2+ diffusion/deposition, suppressing dendrites, improving cycling and reducing energy use and emissions.
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Advancing solar-driven redox processes: pyrene-based covalent organic frameworks for efficient environmental remediation and H2O2 production
DOI: 10.1039/D5GC01711D, PaperA. Yaxuan Zheng, B. Siyu Han, C. Yuxin Sun, D. Zhangpei Chen, E. Yuqiu Huo, F. Jianshe Hu
The rational design of efficient photocatalysts is critical for solar-driven chemical conversions.
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Co-recycling of spent cathode and anode via redox-mediated lithiation
DOI: 10.1039/D5GC02248G, PaperZhimin Du, Peixiang Gao, Yuxiang Chen, Yingming Zhang, Yongzhi Liu, Xuejing Qiu, Lingling Xie
Co-recycling of spent cathode/anode via redox-mediated lithiation enables anodic de-lithiation and cathodic re-lithiation, regenerating Al, Cu, graphite and LiFePO4.
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Catalytic hydrogenolysis of lignin under syngas: the enhancement on the Cβ-O bond cleavage with CO
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC01618E, PaperXinjun He, Mengqiao Gao, Fukun Li, Zhiyang Tang, Jie Qu, Jinxing Long, Qiang Zeng, Xuehui Li
Catalytic hydrogenolysis of lignin has attracted steady attentions in regard of producing high-value aromatic chemicals from the renewable resource and achieving the “carbon neutrality” goal. However, current techniques for lignin...
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DOI: 10.1039/D5GC01618E, PaperXinjun He, Mengqiao Gao, Fukun Li, Zhiyang Tang, Jie Qu, Jinxing Long, Qiang Zeng, Xuehui Li
Catalytic hydrogenolysis of lignin has attracted steady attentions in regard of producing high-value aromatic chemicals from the renewable resource and achieving the “carbon neutrality” goal. However, current techniques for lignin...
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Natural deep eutectic solvents (NaDES): green solvents for pharmaceutical applications and beyond
DOI: 10.1039/D4GC06386D, Critical Review


This review first provides a comprehensive overview of NaDES theory and subsequently explores all potential applications of NaDES in the pharmaceutical industry, highlighting overlooked issues such as toxicity and process limitations.
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Regeneration of iron species for high and stable activity of nickel electrodes in the oxygen evolution reaction
DOI: 10.1039/D5GC00114E, Paper


A regeneration strategy combined with the tuning of traces of iron in the electrolyte enabled achieving high activity and enhanced stability of nickel electrodes in the oxygen evolution reaction (OER).
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Recent advancements in catalytic CO2 conversion to methanol: strategies, innovations, and future directions
DOI: 10.1039/D5GC01906K, Critical ReviewMuhammad Tahir Khalil, Xianli Wu, Shuling Liu, Yanyan Liu, Saima Ashraf, Ruofan Shen, Huanhuan Zhang, Zhikun Peng, Jianchun Jiang, Baojun Li
The catalytic CO2 to methanol conversion enables sustainable fuel production and emissions reduction. Advanced catalysts, reaction mechanisms, and process optimization are critically analyzed.
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